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Mr Black walked around and offered help____we were doing an experiment.

A. while B. although C. until D. unless

A 【解析】句意:布莱克先生在我们做实验的时候在我们身边走来走去提供帮助。A. while正当……时候;B. although尽管;C. until到……为止;D. unless除非,如果不。while与进行时态连用,故答案为A。
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